Observation of Floquet states in graphene

authored by: Marco Merboldt, Michael Schüler, David Schmitt, Jan Philipp Bange, Wiebke Bennecke, Karun Gadge, Klaus Pierz, Hans Werner Schumacher, Davood Momeni, Daniel Steil, Salvatore R. Manmana, Michael Sentef, Marcel Reutzel, Stefan Mathias
Abstract: Recent advances in the field of condensed-matter physics have unlocked the potential to realize and control emergent material phases that do not exist in thermal equilibrium. One of the most promising concepts in this regard is Floquet engineering, the coherent dressing of matter via time-periodic perturbations. However, the broad applicability of Floquet engineering to quantum materials is still unclear. For the paradigmatic case of monolayer graphene, the theoretically predicted Floquet-induced effects, despite a seminal report of the light-induced anomalous Hall effect, have been put into question. Here, we overcome this problem by using electronic structure measurements to provide direct experimental evidence of Floquet engineering in graphene. We report light-matter-dressed Dirac bands by measuring the contribution of Floquet sidebands, Volkov sidebands, and their quantum path interference to graphene's photoemission spectral function. Our results finally demonstrate that Floquet engineering in graphene is possible, paving the way for the experimental realization of the many theoretical proposals on Floquet-engineered band structures and topological phases.
External Organisation(s): University of Göttingen
Paul Scherrer Institut (PSI)
University of Fribourg
Physikalisch-Technische Bundesanstalt PTB
University of Bremen
Center for Free-Electron Laser Science (CFEL)
Type: Preprint
No. of pages: 30
Publication date: 19.04.2024
Publication status: E-pub ahead of print
Electronic version(s): https://doi.org/10.48550/arXiv.2404.12791 (Access: Open)

BibTeX

@techreport{7ad22be882d14b559574a7c43225d7a1,
title = "Observation of Floquet states in graphene",
abstract = " Recent advances in the field of condensed-matter physics have unlocked the potential to realize and control emergent material phases that do not exist in thermal equilibrium. One of the most promising concepts in this regard is Floquet engineering, the coherent dressing of matter via time-periodic perturbations. However, the broad applicability of Floquet engineering to quantum materials is still unclear. For the paradigmatic case of monolayer graphene, the theoretically predicted Floquet-induced effects, despite a seminal report of the light-induced anomalous Hall effect, have been put into question. Here, we overcome this problem by using electronic structure measurements to provide direct experimental evidence of Floquet engineering in graphene. We report light-matter-dressed Dirac bands by measuring the contribution of Floquet sidebands, Volkov sidebands, and their quantum path interference to graphene's photoemission spectral function. Our results finally demonstrate that Floquet engineering in graphene is possible, paving the way for the experimental realization of the many theoretical proposals on Floquet-engineered band structures and topological phases. ",
keywords = "cond-mat.mes-hall",
author = "Marco Merboldt and Michael Sch{\"u}ler and David Schmitt and Bange, {Jan Philipp} and Wiebke Bennecke and Karun Gadge and Klaus Pierz and Schumacher, {Hans Werner} and Davood Momeni and Daniel Steil and Manmana, {Salvatore R.} and Michael Sentef and Marcel Reutzel and Stefan Mathias",
note = "4 main figures, 3 extended figures",
year = "2024",
month = apr,
day = "19",
doi = "10.48550/arXiv.2404.12791",
language = "English",
type = "WorkingPaper",
}