Absorption and multi-phonon quenching in nanocrystal doped SiO2 fibers

authored by
Michael Steinke, Simon Spelthann, Axel Rühl, Detlev Ristau
Abstract

SiO

2 fibers doped with rare-earth-doped nanocrystals are promising to overcome the strong SiO

2 multi-phonon quenching and could yield novel laser gain materials. So far, no attention has been paid to the question how well the nanocrystals can suppress the quenching depending on the properties of the SiO

2 host glass. Here, a novel analytical model was applied to study the impact of the glass purity and composition on the quenching efficiency. Only a few experimentally accessible material and design parameters are required to compute the average quenching rate inside the nanocrystals. It is demonstrated that sufficiently low levels of quenching can only be expected for SiO

2 free of impurities or dopants that increase the multi-phonon absorption. This indicates that high-purity aluminosilicate glasses, in contrast to phosphosilicate and borosilicate glasses, are ideal hosts.

Organisation(s)
Institute of Quantum Optics
QUEST-Leibniz Research School
PhoenixD: Photonics, Optics, and Engineering - Innovation Across Disciplines
QuantumFrontiers
External Organisation(s)
Laser Zentrum Hannover e.V. (LZH)
Type
Article
Journal
Optical materials express
Volume
11
Pages
1631-1642
No. of pages
12
ISSN
2159-3930
Publication date
06.2021
Publication status
Published
Peer reviewed
Yes
ASJC Scopus subject areas
Electronic, Optical and Magnetic Materials
Electronic version(s)
https://doi.org/10.1364/OME.424116 (Access: Open)